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Mapping dynamical heterogeneity in structural glasses to correlated fluctuations of the time variables

机译:将结构玻璃中的动态异质性映射到相关的   时间变量的波动

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摘要

Dynamical heterogeneities -- strong fluctuations near the glass transition --are believed to be crucial to explain much of the glass transitionphenomenology. One possible hypothesis for their origin is that they emergefrom soft (Goldstone) modes associated with a broken continuous symmetry undertime reparametrizations. To test this hypothesis, we use numerical simulationdata from four glass-forming models to construct coarse grained observablesthat probe the dynamical heterogeneity, and decompose the fluctuations of theseobservables into two transverse components associated with the postulatedtime-fluctuation soft modes and a longitudinal component unrelated to them. Wefind that as temperature is lowered and timescales are increased, the timereparametrization fluctuations become increasingly dominant, and that theircorrelation volumes grow together with the correlation volumes of the dynamicalheterogeneities, while the correlation volumes for longitudinal fluctuationsremain small.
机译:动态异质性-玻璃化转变附近的剧烈波动-被认为对于解释许多玻璃化转变现象至关重要。关于其起源的一种可能的假设是,它们从与破坏的连续对称性重新定型相关联的软(金石)模式中出现。为了检验该假设,我们使用来自四个玻璃成形模型的数值模拟数据来构造粗糙的可观察物,以探测动态异质性,并将这些可观察物的波动分解为与假定的时间波动软模相关的两个横向分量以及与它们无关的纵向分量。 。我们发现,随着温度的降低和时间尺度的增加,时间重新参数化波动变得越来越占主导地位,并且它们的相关量与动态异质性的相关量一起增长,而纵向波动的相关量仍然很小。

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